Definitely Portal.. that game is simply mind-blowing in the hundred's of ways that you can work around the obstacles.. just to find out the cake is a lie.. Sticking to FPSs, Mirror's Edge made use of an intriguing graphics engine and... well, it's a game where you can parkour in first person for Pete's sake! I'd add Crush for the PSP; I generally believe that puzzle games are more prone to innovation..
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