Not sure what exactly you're after so I'll add 2.5D games in too and basically make it a list of games which play in a 16-bit style
Castlevania Symphony of the Night - needs no introduction
Alundra - Very good Link to the Past ripoff
Gunners Heaven - Gunstar Heroes style game - import only
Oddworld series
Adventures of Lomax - very difficult platformer starring a lemming
Buster Bros Collection - a kind of shmup where you fire up at bubbles which split into more bubbles when shot (better than it sounds)
Mega Man series
Rayman
R-Type's
R-Type Delta
Silhouette Mirage
Strider 2 - awesome
Tomba series
Klonoa
Einhander
G-Darius
Wild 9 - weird grapple hook platformer made by Earthworm Jim people
Thunder Force V - Better on Saturn but the PS1 version is still excellent - Import only
Legend of Mana
In the Hunt - submarine shmup
Don Pachi Series - Import only
Lunar series - great 16-bit style RPG's
Breath of Fire 3
The Final Fantasy remakes
Norse by Northwest - Lost Vikings sequel
Street Fighter Alpha 3
Metal Slug X
Suikoden Series
Super Puzzle Fighter 2
Darkstalkers 3
Strikers 1945
Thats what I can think of at the moment, but there's so many that its hard to remember them all, and there's such a huge amount of PS1 games that there's still a lot I've yet to play (especially imports)
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