A nice long one is FFIII.... but it's $16!!!! If you don't mind shelling out that much, then it's one I'd recommend. It'll take about 40-50 hrs to finish. If you haven't yet, perhaps you can use part of the $25 credit which you should have received with your N7.
Max Payne I believe is about 8 or so hours, I'm not sure if you consider that lengthy.
GTA III should also take you some time. I heard though that due to the way the controls are set up, it's fine to screw around the city, but difficult for actually playing through the campaign.
For non-ports, Castle Master 3D is fun. It gets quite difficult quickly, especially when the AI decided to attack you from all sides. It's kind of like Risk with RPG elements and a bit of Dynasty Warrior.
ZDefense also took up a bit of my time, but you might consider it a casual game. The game comes with quite abit of maps, and you can download a few more which should take you 30+ hrs to complete all. I thought I was done with TD, but I got pretty obsessed with this game.
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