I think Call of Duty 4, because it got better reviews, the missions last pretty long (15-20 minutes each), there are a few more weapons, and it has a pretty good framerate for the most part.
But I've never played Brothers in Arms, so I don't have an opinion on that one. :D
If you want the one that is longer, get Call of Duty 4. If you care more about a more memorable experience and better graphics/ production, get Brothers in Arms.
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