You need both a Gamecube controller and a memory card. Also, the Wii will act as a GameCube. So the wiimote will be useless on the GameCube games likeyou can't press on the home button during a game.
What happens is that the console basically switches it's hardware to "Gamecube yo", so no Wii-specific features will work. This includes bluetooth (for your wiimote) and HDD access.
So in order to play GCN games, you need GCN controllers and memory cards.
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