iOS > Android
Both are incredibly similar in terms of functionality but I prefer iOS. It is smoother, more responsive and much more intuitive. It never lags or crashes and its performance is unified since it runs on specific devices. Android on the top spec Android phone is good, but its awful on the mid range products.
The Android market is too fragmented and as a result its an unreliable format. Every Android phone I've used with few exceptions (the top spec ones) are sluggish and unresponsive. The top spec ones are comparable to iOS but they still lack the smoothness.
Hardware wise the iPhone is what propels iOS ahead. The iPhone touch screen is still the best and creates the best user experience, and the Retina Displays blows all the others out of the water. iPhone battery life is still miles ahead of Android phones too. The App Store is still the best place to get apps as well.
Conclusion - Both are good but iOS is still on top.
I left out WP7 since I have not used it yet.
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