BF3 is good for any reason an FPS is fun to play online, and it also does well with the various vahicles.
A couple PC-exclusives that I've had a lot of fun with:
1) Tribes: Ascend is a free-to-play FPS that's well worth the time to download.
2) Ravaged, which is a 'post-apocalyptic' FPS (also third-person view) with all the standard modes.
Not sure if it's free on any console, but on PC, Team Fortress 2 is also free to play and is still fairly active.
For multiplats that are also fun multiplayer, you have Crysis 2 and 3 which are also different-enough from Call of Duty thanks to the varied maps and the suit powers.
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