Hm. Where to begin?
FPS:
Doom, Doom 2 and Final Doom
System Shock 2
Deus Ex
Tron 2.0
Call of Duty
Quake 2 and Quake 3
Half Life
Rogue Spear
Brothers in Arms Road to Hill 30 and Earned in Blood
Aliens vs Predator
No One Lives Forever
Half Life 2 if you can run Source games
RTS:
Medieval Total War
Dawn of War
Command and Conquer The First Decade
RPG:
Fallout
Fallout 2
Planescape Torment
Baldur's Gate
Baldur's Gate 2
Diablo 2
Vampire the Masquerade Bloodlines if you can run Source games
Icewind Dale
Neverwinter Nights
Other:
Broken Sword 1-3
Sam and Max Hit the Road, Season 1 and Season 2
Any Monkey Island games you can find
Grim Fandango
Myst series
The entire Grand Theft Auto series
Alpha Centauri
Aquaria
Splinter Cell and Pandora Tomorrow
I'm sure I'm missing plenty, but as you can see there is no shortage of excellent games available for you to play - indeed, most of the best games the PC has ever seen are pre-2000. Many of the above also have expansions.
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