If you are talking about specifically for the PlayStation 2, then I would have to say Mortal Komat: Armageddon. It was the worst game in terms of storyline and extras, but the gameplay was the most refined and I think it played the best out of Deadly Alliance, Deception and itself.
I have a really strong attachement to Deadly Alliance for some reason though. The intro movie is fantastic and the voice actor for Raiden did a really good job. I also love the fact that it was the first (really good) 3D Mortal Kombat game and it had a lot of the original old-school characters, and it just had this really cool feeling about it. Although it does have some noticeable flaws however.
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