I'd be guessing the 360 version, simply because the machine is more powerful and the controller has more buttons. I remember the GS review saying that the games were pretty close though. For more details you might want to look up the PSP review.
If it means a lot to you, you might want to look in the difference in characters. The PSP has a few not available on the 360 and vice versa. I know hawkeye is psp exclusive and moon knight is on the 360. There are a few more but I can remember em right now.Â
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