My favorite ever is from Quake 4, with World of Padman (the full version in the game though is much better), StarFox Assault and Star Trek: Deep Space Nine - The Fallen in runner-up positions. The most notable themes for me (in games that have ambient-to-no actual menu music) are from Crysis, Descent 3 (too bad the rest of the game completely sucked), and Return to Castle Wolfenstein.
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