I would have to emulate the suggestion of S.T.A.L.K.E.R and make mention that I enjoyed it the most when I wasn't following the story missions, the world truly breathes around you.
Some other games outside of the FPS realm that keep with the spirit of DEUS EX (that whole, hah told you that you could merge two different gaming genres succesfully spirit) are Planescape Torment, Baldurs Gate Series, and Fallout Series (tactical RPG). Also in that spirit the recent UFO games, though rough in their presentation can be real gems.
I hesitate to recommend BIOSHOCK as I have found it wanting compared to System Shock 2, but games that have a more immersive flair than the aforementioned isometric RPG's are Indigo Prophecy, Dark Messiah of M&M (have to be forgiving of its shortcomings, but can be fairly enjoyable), and if you are a fan of open ended sprawling try out Morrowind - though Oblivion may have better graphics and more streamlined gameplay Morrowind is massive with all of the user created additions and add-ons, and it is fairly inexpensive.
But last but certainly not least, if you are willing to look way back into the gaming golden age, some of my favorites are Eye of the Beholder 1-3, Might and Magic 4,5,6... 7 is ok. Wow, sorry for the long post.
Cheers
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