I'm going to go with MGS3. I liked its story the most, and I think Kojima balanced the cinematics with the game-play the best. On top of that, the bosses were so memorable for me. Before I learned a few tricks for beating The End, I had a two-hour fight with him. Despite that length of the battle, there was no frustration. Truly unforgettable!
I just got it as my first game for Xbox 360, and what a way to start off in this generation of gaming. I was totally enthralled right until the end, and I started back into it immediately. I love how polished it is.
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