tough one, a bunch of games spring top mind -
dragon's lair - not so much a game as a cartoon with interactive moments though.
the original prince of persia - at the time had super realistic character animations that were much better than anything seen before, created using some painstakingly manual illustration based technique iirc.
another world - incredible intro and overall beautifully stylish game.
the arcade port of streetfighter 2 on the snes. mind blowing at the time.
the secret of monkey island 2. the first was beautiful, the second though was something else entirely.
the original star fox, mode 7 ftw
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