I doubt you even need to play MGS3, just MGS2. However, I would definitely recommend the MGS Essential Collection, because MGS2 and 3 are two of the greatest games ever made (along with 1). Without spoiling anything, I will just tell you that MGS3 takes place before 1 and 2, and really just answers a lot of questions and offers insight to the events that happen in 1 and 2.
MGS4 takes place after MGS2. MGS: PO is a great game, and takes place 6 years after MGS3, but still long before MGS2. MGS: PO (and it's sequel) is probably the least necessary of the MGS games you need to play, not counting MG Acid. However, it is good, so if you can find it for a decent price, you may wanna play it anyway. I would definitely recommend 2 and 3 over PO though.
edit: err, I see you said you were gonna play MGS2 and 3, nevermind. ;) Enjoy, I'm sure you will.
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