The imidiate thing that jumps into my eyes are that The Punisher is very well fit for a game, unlike some of the others, He is human, and he IS violent. So if you look at it from possible gameplay he would be the easiest.
I suppose The crow is also fairly easy to make a decent game over, seeing as he is a vengeful (insert word here) that thends to like sharp stabby objects and guns. And that game would atleast have a justified health regen setting :P
These are if we look at what games are, if they can pose a challange, and if they have the right team.
The more difficult one would be superman, he is pretty much invinsible so you could not make a fun game about him, unless you took liberties. It can surely be done, but we would likely see devs looking outside conventional videogame buildups to make such a game a hit (and more importantly a good one)
With the right team of devs (who also happen to be real fans) anyone can have a great game, I just pick the two above, because they would be Easiest to make a game for, since they sort of fit into gaming as it is without much hassle.
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