First off, DO NOT BUY ELF BOWLING.
Secondly, you should realize that good story and Wifi don't really go hand in hand.
Hotel Dusk has a great story, if you don't mind a more relaxed game. Just don't expect it to get your blood going like a true action game.
RPGs like Final Fantasy III probably have good stories too although they can also be too difficult for some players' likings.
As for Wifi, look to games with a large following, so that you can find many opponents quickly and easily. The games with the most online players seem to be Mario Kart, Metroid Prime, Tetris, and a few others. What you need to beware of are games lke Clubhouse games, because while it still has a pretty good online mode, you can only find opponents regularly for about 10 of its 35 wifi games, simply because not enough people want to play games like chinese checkers or hangman for oppenents to pair up.
 good luck!
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